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1 article(s) from Sharma, Nidhi

Synthesis and optoelectronic properties of benzoquinone-based donor–acceptor compounds

Daniel R. Sutherland,
Nidhi Sharma,
Georgina M. Rosair,
Ifor D. W. Samuel,
Ai-Lan Lee and
Eli Zysman-Colman

Beilstein J. Org. Chem. 2019, 15, 2914–2921, doi:10.3762/bjoc.15.285

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Scheme 1: Mild and direct C–H monofunctionalization of BQ 1: previous [14] and this work.

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Figure 1: Benzoquinone derivatives synthesized for this study, with the donor in red and the benzoquinone acc...

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Scheme 2: Synthesis of 2–4 via mild and direct C–H monofunctionalization of BQ (1).

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Scheme 3: Synthesis of 5 via double Suzuki coupling.

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Figure 2: Crystal structures of 3 and 4.

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Figure 3: HOMO/LUMO and S₁/T₁ energies as well as HOMO/LUMO electron density distribution profiles of 2–5.

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Figure 4: Cyclic voltammograms and differential pulse voltammograms of 2–5 in degassed DCM (scan rate = 100 m...

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Figure 5: UV–vis absorption spectra of 2–5 in DCM and photoluminescence spectrum of 3 in degassed DCM and in ...

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Figure 6: Time-resolved PL plots. a) Prompt decay and b) delayed decay curve of 3 in thin film (λ_exc = 378 nm...

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Published 04 Dec 2019

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